Researchers achieve atomic-scale control of quantum interference

Electric control of the energy detuning of a single Ti spin. Credit: Nature Communications (2025). DOI: 10.1038/s41467-025-64022-9

In a study published in Nature Communications, a research team demonstrates the all-electrical control of quantum interference in individual atomic spins on a surface.

Quantum interference arises when a system exists in a superposition of states, with relative phases producing constructive or destructive interference. An example is Landau-Zener-Stückelberg-Majorana (LZSM) interference, which arises when a quantum two-level system is repeatedly driven through an anticrossing in the energy-level diagram, and undergoes multiple nonadiabatic transitions.

This mechanism is a powerful tool for fast and reliable quantum control, but it remains a significant challenge to achieve tunable LZSM interference in an atomic-scale quantum architecture where multiple spins can be precisely assembled and controllably coupled on demand.

In this study, using a custom-built advanced microscope known as electron spin resonance-scanning tunneling microscope (ESR-STM), the researchers developed an all-electrical method to control LZSM quantum interference in individual and coupled atomic spins on insulating films.

By modulating atomically confined tip-atom interactions with strong electric fields, they rapidly drove spin states through anticrossings and observed rich interference patterns, including multiphoton resonances and signatures of spin-transfer torque.

Multilevel LZSM spectra measured on coupled spins with tunable interactions showed distinct interference patterns depending on their many-body energy landscapes.

These findings open new avenues for all-electrical quantum manipulation in spin-based quantum processors in the strongly driven regime. This study opens up new possibilities for fast and robust quantum-state manipulation at the atomic scale.

The researchers were led by Prof. Yang Kai from the Institute of Physics of the Chinese Academy of Sciences, along with Prof. Joaquín Fernández-Rossier from International Iberian Nanotechnology Laboratory.

More information:
Hao Wang et al, Electrically tunable quantum interference of atomic spins on surfaces, Nature Communications (2025). DOI: 10.1038/s41467-025-64022-9

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Chinese Academy of Sciences

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Researchers achieve atomic-scale control of quantum interference (2025, October 14)
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