Reinsel, D., Gantz, J. & Rydning, J. The digitization of the world from edge to core White Paper No. US44413318 (IDC, 2018) https://www.seagate.com/files/www-content/our-story/trends/files/idc-seagate-dataage-whitepaper.pdf

Archival disc technology White Paper (Sony and Panasonic, 2020) https://panasonic.cn/wp-content/uploads/2020/05/Archival-Disc-Technology-%EF%BC%9A2nd-Edition.pdf

DeBoer, S. The future of the national semiconductor technology center. Micron https://www.micron.com/about/blog/2022/august/micron-and-western-digital (2022).

Microsoft Research Project Silica Team Laser writing in glass for dense, fast and efficient archival data storage. Nature 650, 606–612 (2026).

Article 
ADS 

Google Scholar
 

Gu, M., Li, X. & Cao, Y. Optical storage arrays: a perspective for future big data storage. Light Sci. Appl. 3, e177 (2014).

Article 
ADS 

Google Scholar
 

Lamon, S., Zhang, Q. & Gu, M. Nanophotonics-enabled optical data storage in the age of machine learning. APL Photonics 6, 110902 (2021).

Article 
ADS 

Google Scholar
 

Lamon, S., Zhang, Q., Yu, H. & Gu, M. Neuromorphic optical data storage enabled by nanophotonics: a perspective. ACS Photonics 11, 874–891 (2024).

Article 

Google Scholar
 

Bruder, F., Hagen, R., Rölle, T., Weiser, M. & Fäcke, T. From the surface to volume: concepts for the next generation of optical-holographic data-storage materials. Angew. Chem. Int. Ed. 50, 4552–4573 (2011).

Article 

Google Scholar
 

Smith, M. Ultra HD Blu-ray format video characteristics. SMPTE Motion Imaging J. 125, 14–27 (2016).

Article 

Google Scholar
 

Parthenopoulos, D. & Rentzepis, P. Three-dimensional optical storage memory. Science 245, 843–845 (1989).

Article 
ADS 

Google Scholar
 

Strickler, J. & Webb, W. Three-dimensional optical data storage in refractive media by two-photon point excitation. Opt. Lett. 16, 1780–1782 (1991).

Article 
ADS 

Google Scholar
 

Ryan, C. et al. Roll-to-roll fabrication of multilayer films for high capacity optical data storage. Adv. Mater. 24, 5222–5226 (2012).

Article 

Google Scholar
 

Grotjohann, T. et al. Diffraction-unlimited all-optical imaging and writing with a photochromic GFP. Nature 478, 204–208 (2011).

Article 
ADS 

Google Scholar
 

Li, X., Cao, Y., Tian, N., Fu, L. & Gu, M. Multifocal optical nanoscopy for big data recording at 30 TB capacity and gigabits/second data rate. Optica 2, 567–570 (2015).

Article 
ADS 

Google Scholar
 

Lamon, S., Wu, Y., Zhang, Q., Liu, X. & Gu, M. Nanoscale optical writing through upconversion resonance energy transfer. Sci. Adv. 7, eabe2209 (2021).

Article 
ADS 

Google Scholar
 

Zhao, M. et al. A 3D nanoscale optical disk memory with petabit capacity. Nature 626, 772–778 (2024).

Article 
ADS 

Google Scholar
 

Zhou, J. et al. Terabit-scale high-fidelity diamond data storage. Nat. Photonics 18, 1327–1334 (2024).

Article 
ADS 

Google Scholar
 

Goda, A. Recent progress on 3D NAND flash technologies. Electronics 10, 3156 (2021).

Article 

Google Scholar
 

Wuttig, M. & Yamada, N. Phase-change materials for rewriteable data storage. Nat. Mater. 6, 824–832 (2007).

Article 

Google Scholar
 

Zhang, J., Gecevičius, M., Beresna, M. & Kazansky, P. Seemingly unlimited lifetime data storage in nanostructured glass. Phys. Rev. Lett. 112, 033901 (2014).

Article 
ADS 

Google Scholar
 

Gao, J. et al. Multi-dimensional shingled optical recording by nanostructuring in glass. Adv. Funct. Mater. 34, 2306870 (2024).

Article 

Google Scholar
 

Zijlstra, P., Chon, J. & Gu, M. Five-dimensional optical recording mediated by surface plasmons in gold nanorods. Nature 459, 410–413 (2009).

Article 
ADS 

Google Scholar
 

Ouyang, X. et al. Synthetic helical dichroism for six-dimensional optical orbital angular momentum multiplexing. Nat. Photonics 15, 901–907 (2021).

Article 
ADS 

Google Scholar
 

Kallepalli, D. et al. Ultra-high density optical data storage in common transparent plastics. Sci. Rep. 6, 26163 (2016).

Article 
ADS 

Google Scholar
 

Shen, Y., Le, X., Wu, Y. & Chen, T. Stimulus-responsive polymer materials toward multi-mode and multi-level information anti-counterfeiting: recent advances and future challenges. Chem. Soc. Rev. 53, 606–623 (2024).

Article 

Google Scholar
 

Auzel, F. Upconversion and anti-Stokes processes with f and d ions in solids. Chem. Rev. 104, 139–174 (2004).

Article 

Google Scholar
 

Liu, X., Yan, C. & Capobianco, J. Photon upconversion nanomaterials. Chem. Soc. Rev. 44, 1299–1301 (2015).

Article 

Google Scholar
 

Richards, B., Hudry, D., Busko, D., Turshatov, A. & Howard, I. Photon upconversion for photovoltaics and photocatalysis: a critical review. Chem. Rev. 121, 9165–9195 (2021).

Article 

Google Scholar
 

Zhang, C. et al. Luminescence modulation of ordered upconversion nanopatterns by a photochromic diarylethene: rewritable optical storage with nondestructive readout. Adv. Mater. 22, 633–637 (2010).

Article 

Google Scholar
 

Zheng, K. et al. Rewritable optical memory through high-registry orthogonal upconversion. Adv. Mater. 30, 1801726 (2018).

Article 

Google Scholar
 

Lamon, S., Wu, Y., Zhang, Q., Liu, X. & Gu, M. Millisecond-timescale, high-efficiency modulation of upconversion luminescence by photochemically derived graphene. Adv. Opt. Mater. 7, 1901345 (2019).

Article 

Google Scholar
 

Gu, W. et al. Thermo-optical sub-micrometer ultrahigh luminescence emission tuning in hybrid organic-inorganic upconversion nanocomposites for data storage and anticounterfeiting. Adv. Opt. Mater. 13, 2402248 (2025).

Article 

Google Scholar
 

Lu, Y. et al. Tunable lifetime multiplexing using luminescent nanocrystals. Nat. Photonics 8, 32–36 (2014).

Article 
ADS 

Google Scholar
 

Lee, C. et al. Indefinite and bidirectional near-infrared nanocrystal photoswitching. Nature 618, 951–958 (2023).

Article 
ADS 

Google Scholar
 

Gu, W. et al. Topology-driven energy transfer networks for upconversion stimulated emission depletion microscopy. Light Sci. Appl. 14, 395 (2025).

Article 
ADS 

Google Scholar
 

Zhang, H. et al. Time-tuned photon avalanche upconversion in nanoparticles for optical logic and multidimensional data encoding. ACS Photonics 13, 1477–1491 (2026).

Article 

Google Scholar
 

Wen, S. et al. Advances in highly doped upconversion nanoparticles. Nat. Commun. 9, 2415 (2018).

Article 
ADS 

Google Scholar
 

Lamon, S., Yu, H., Zhang, Q. & Gu, M. Lanthanide ion-doped upconversion nanoparticles for low-energy super-resolution applications. Light Sci. Appl. 13, 252 (2024).

Article 
ADS 

Google Scholar
 

Xia, C., Zhu, S., Feng, T., Yang, M. & Yang, B. Evolution and synthesis of carbon dots: from carbon dots to carbonized polymer dots. Adv. Sci. 6, 1901316 (2019).

Article 

Google Scholar
 

Xia, C. et al. The formation mechanism of carbonized polymer dots: cross-linking-induced nucleation and carbonization. Angew. Chem. Int. Ed. 63, e202410519 (2024).

Article 

Google Scholar
 

Tao, S. et al. Confined-domain crosslink-enhanced emission effect in carbonized polymer dots. Light Sci. Appl. 11, 56 (2022).

Article 
ADS 

Google Scholar
 

Li, P. & Sun, Z. An innovative way to modulate the photoluminescence of carbonized polymer dots. Light Sci. Appl. 11, 81 (2022).

Article 
ADS 

Google Scholar
 

Zheng, C. et al. Crosslink-enhanced emission-dominated design strategy for constructing self-protective carbonized polymer dots with near-infrared room-temperature phosphorescence. Angew. Chem. Int. Ed. 63, e202408516 (2024).

Article 

Google Scholar
 

Wang, Y. et al. Dye-incorporated carbonized polymer dots with tunable solid-state emission based on intraparticle Förster resonance energy transfer. Adv. Funct. Mater. 34, 2402825 (2024).

Article 

Google Scholar
 

Wang, Z. et al. Gram-scale synthesis of 41% efficient single-component white-light-emissive carbonized polymer dots with hybrid fluorescence/phosphorescence for white light-emitting diodes. Adv. Sci. 7, 1902688 (2020).

Article 

Google Scholar
 

Kang, C. et al. Enabling carbonized polymer dots with color-tunable time-dependent room temperature phosphorescence through confining carboxyl dimer association. Angew. Chem. Int. Ed. 136, e202316527 (2024).

Article 

Google Scholar
 

Shen, Y. et al. High-temperature resistance photoluminescence carbonized polymer dots through equilibrium bi-confinement effects. Adv. Mater. 37, 2407811 (2025).

Wang, Y. et al. The synthesis of functionalized carbonized polymer dots via reversible assembly of oligomers for anti-counterfeiting, catalysis, and gas storage. Adv. Sci. 11, 2405043 (2024).

Article 

Google Scholar
 

Sugioka, K. & Cheng, Y. Ultrafast lasers–reliable tools for advanced materials processing. Light Sci. Appl. 3, e149 (2014).

Article 
ADS 

Google Scholar
 

Malinauskas, M. et al. Ultrafast laser processing of materials: from science to industry. Light Sci. Appl. 5, e16133 (2016).

Article 
ADS 

Google Scholar
 

Gardner, T. Has HDD areal density stalled? StorageNewsletter https://www.storagenewsletter.com/2022/04/19/has-hdd-areal-density-stalled (2022).

Ge, Q. et al. 3D printing of highly stretchable hydrogel with diverse UV curable polymers. Sci. Adv. 7, eaba4261 (2021).

Article 
ADS 

Google Scholar
 

Zhang, M. et al. Micro-and nanofabrication of dynamic hydrogels with multichannel information. Nat. Commun. 14, 8208 (2023).

Article 
ADS 

Google Scholar
 

Loh, K., Bao, Q., Eda, G. & Chhowalla, M. Graphene oxide as a chemically tunable platform for optical applications. Nat. Chem. 2, 1015–1024 (2010).

Article 

Google Scholar
 

Crochet, J., Duque, J., Werner, J. & Doorn, S. Photoluminescence imaging of electronic-impurity-induced exciton quenching in single-walled carbon nanotubes. Nat. Nanotechnol. 7, 126–132 (2012).

Article 
ADS 

Google Scholar
 

Cheng, Q. et al. Recent advances in optical technologies for data centers: a review. Optica 5, 1354–1370 (2018).

Article 
ADS 

Google Scholar
 

You, R. et al. Laser fabrication of graphene-based flexible electronics. Adv. Mater. 32, 1901981 (2020).

Article 

Google Scholar
 

Devi, M., Wang, H., Moon, S., Sharma, S. & Strauss, V. Laser carbonization–a powerful tool for micro-fabrication of patterned electronic carbons. Adv. Mater. 35, 2211054 (2023).

Article 

Google Scholar
 

Wang, Z. et al. Thermally driven amorphous-crystalline phase transition of carbonized polymer dots for multicolor room-temperature phosphorescence. Adv. Opt. Mater. 9, 2100421 (2021).

Article 

Google Scholar
 

Liu, Y., Zheng, C. & Yang, B. Phosphorus and nitrogen codoped carbonized polymer dots with multicolor room temperature phosphorescence for anticounterfeiting painting. Langmuir 38, 8304–8311 (2022).

Article 

Google Scholar
 

Zhang, Q., Xu, S., Zhang, L., Yang, L. & Jiang, C. Multiemitting ultralong phosphorescent carbonized polymer dots via synergistic enhancement structure design. Adv. Sci. 11, 2400781 (2024).

Article 

Google Scholar
 

Akizuki, N., Aota, S., Mouri, S., Matsuda, K. & Miyauchi, Y. Efficient near-infrared up-conversion photoluminescence in carbon nanotubes. Nat. Commun. 6, 8920 (2015).

Article 
ADS 

Google Scholar
 

Jones, A. et al. Excitonic luminescence upconversion in a two-dimensional semiconductor. Nat. Phys. 12, 323–327 (2016).

Article 

Google Scholar
 

Jadczak, J. et al. Room temperature multi-phonon upconversion photo-luminescence in monolayer semiconductor WS2. Nat. Commun. 10, 107 (2019).

Article 
ADS 

Google Scholar
 

Qi, P. et al. Giant excitonic upconverted emission from two-dimensional semiconductor in doubly resonant plasmonic nanocavity. Light Sci. Appl. 11, 176 (2022).

Article 
ADS 

Google Scholar
 

Dai, Y. et al. Phonon-assisted upconversion in twisted two-dimensional semiconductors. Light Sci. Appl. 12, 6 (2023).

Article 
ADS 

Google Scholar
 

Tran, T. et al. Anti-Stokes excitation of solid-state quantum emitters for nanoscale thermometry. Sci. Adv. 5, eaav9180 (2019).

Article 
ADS 

Google Scholar
 

Ye, Z. et al. Phonon-assisted up-conversion photoluminescence of quantum dots. Nat. Commun. 12, 4283 (2021).

Article 
ADS 

Google Scholar
 

Qiu, X. et al. Near-Infrared upconversion luminescence and bioimaging in vivo based on quantum dots. Adv. Sci. 6, 1801834 (2019).

Article 

Google Scholar
 

Wu, B. et al. Uncovering the mechanisms of efficient upconversion in two-dimensional perovskites with anti-Stokes shift up to 220 meV. Sci. Adv. 9, eadi9347 (2023).

Article 

Google Scholar
 

Gao, C. et al. Application of triplet-triplet annihilation upconversion in organic optoelectronic devices: advances and perspectives. Adv. Mater. 33, 2100704 (2021).

Article 
ADS 

Google Scholar
 

Uji, M., Zähringer, T., Kerzig, C. & Yanai, N. Visible-to-UV photon upconversion: recent progress in new materials and applications. Angew. Chem. Int. Ed. 62, e202301506 (2023).

Article 

Google Scholar
 

Gu, W. et al. Femtosecond laser melting upconversion nanoparticles for sub-micrometer optical patterning. Opt. Express 33, 16317–16327 (2025).

Article 
ADS 

Google Scholar