{"id":249191,"date":"2025-10-30T02:43:16","date_gmt":"2025-10-30T02:43:16","guid":{"rendered":"https:\/\/www.newsbeep.com\/ca\/249191\/"},"modified":"2025-10-30T02:43:16","modified_gmt":"2025-10-30T02:43:16","slug":"spin-environment-of-a-superconducting-qubit-in-high-magnetic-fields","status":"publish","type":"post","link":"https:\/\/www.newsbeep.com\/ca\/249191\/","title":{"rendered":"Spin environment of a superconducting qubit in high magnetic fields"},"content":{"rendered":"<p>In Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1<\/a> we present the field resilient gralmonium qubit, fabricated from a single layer of grAl (cf. Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1a<\/a>), with a critical field on the order of Bc\u2009~\u20096\u2009T<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 39\" title=\"Borisov, K. et al. Superconducting granular aluminum resonators resilient to magnetic fields up to 1 Tesla. Appl. Phys. Lett. 117, &#010;                  https:\/\/doi.org\/10.1063\/5.0018012&#010;                  &#010;                 (2020).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR39\" id=\"ref-link-section-d54651764e747\" rel=\"nofollow noopener\" target=\"_blank\">39<\/a>. We use a 20\u2009nm thick grAl film with a sheet inductance of L\u25a1\u2009=\u20090.75\u2009nH\/\u25a1 (resistivity \u03c1\u2009=\u20092000\u2009\u03bc\u03a9\u2009cm) to design all circuit elements (cf. \u201cMethods\u201d). We galvanically couple a 1\u2009mm long stripline readout resonator to the qubit circuit, consisting of a superinductor, a geometric finger capacitance and a grAl nanojunction. Implemented by a \u00a0~(20\u2009nm)3 grAl volume, the nanojunction offers a sinusoidal current-phase relation similar to conventional Al\/AlOx\/Al JJ<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 46\" title=\"Rieger, D. et al. Granular aluminium nanojunction fluxonium qubit. Nat. Mater. 22, 194 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR46\" id=\"ref-link-section-d54651764e765\" rel=\"nofollow noopener\" target=\"_blank\">46<\/a>, while exposing a minute cross-section to Fraunhofer interference. To reduce the sensitivity to magnetic flux fluctuations perpendicular to the thin film, we implement a gradiometric design<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 48\" title=\"Gusenkova, D. et al. Operating in a deep underground facility improves the locking of gradiometric fluxonium qubits at the sweet spots. Appl. Phys. Lett. 120, &#010;                  https:\/\/doi.org\/10.1063\/5.0075909&#010;                  &#010;                 (2022).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR48\" id=\"ref-link-section-d54651764e769\" rel=\"nofollow noopener\" target=\"_blank\">48<\/a> with two flux loops (ocher &amp; violet in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1a<\/a>) containing fluxes \u03a61,\u00a0\u03a62, respectively. The equivalent circuit diagram in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1b<\/a> can be mapped to the standard fluxonium Hamiltonian<\/p>\n<p>$$H=4{E}_{{{\\rm{C}}}}{\\hat{n}}^{2}+\\frac{1}{2}{E}_{{{\\rm{L}}}}{\\left(\\hat{\\varphi }-2\\pi \\frac{{\\Phi }_{{{\\rm{ext}}}}}{{\\Phi }_{0}}\\right)}^{2}-{E}_{{{\\rm{J}}}}\\cos \\hat{\\varphi }\\,,$$<\/p>\n<p>\n                    (1)\n                <\/p>\n<p>where \\({E}_{{{\\rm{L}}}}={({\\Phi }_{0}\/2\\pi )}^{2}\/{L}_{{{\\rm{q}}}}\\), EC\u2009=\u2009e2\/2C, EJ\u2009=\u2009Ic\u03a60\/2\u03c0 and \u03a60\u2009=\u2009h\/2e. Here, \\(\\hat{n}\\) represents the number of Cooper pairs and \\(\\hat{\\varphi }\\) is the phase difference across the junction. Due to the low intrinsic capacitance of the nanojunction, the qubit charging energy EC is dominated by the interdigitated capacitor C<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 46\" title=\"Rieger, D. et al. Granular aluminium nanojunction fluxonium qubit. Nat. Mater. 22, 194 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR46\" id=\"ref-link-section-d54651764e1171\" rel=\"nofollow noopener\" target=\"_blank\">46<\/a>. For the gradiometric circuit, the effective qubit inductance is given by \\({L}_{{{\\rm{q}}}}=\\frac{{L}_{1,{{\\rm{s}}}}{L}_{2}+{L}_{2}{L}_{3}+{L}_{3}{L}_{1,{{\\rm{s}}}}}{{L}_{1,{{\\rm{s}}}}+{L}_{3}}\\) with L1,s\u2009=\u2009L1\u2009+\u2009Ls, and the effective external flux is<\/p>\n<p>$${\\Phi }_{{{\\rm{ext}}}}={\\Phi }_{\\Delta }-\\alpha {\\Phi }_{\\Sigma }\\,.$$<\/p>\n<p>\n                    (2)\n                <\/p>\n<p>Here, \\({\\Phi }_{\\Sigma \/\\Delta }=\\frac{{\\Phi }_{{{\\rm{ext,1}}}}}{2}\\pm \\frac{{\\Phi }_{{{\\rm{ext,2}}}}}{2}\\) denote the mean and difference of fluxes in the two loops, respectively, and \\(\\alpha=\\frac{{L}_{1,{{\\rm{s}}}}-{L}_{3}}{{L}_{1,{{\\rm{s}}}}+{L}_{3}}\\) is the inductance asymmetry. In our gradiometric design, the magnetic flux susceptibility is reduced by a factor of \u03a6ext,1\/\u03a6\u0394\u2009=\u20094.6 with \u03b1\u2009\u2248\u20090 (cf. Supplementary <a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">II<\/a>).<\/p>\n<p>Fig. 1: Gradiometric gralmonium qubit resilient to Tesla magnetic field.<a class=\"c-article-section__figure-link\" data-test=\"img-link\" data-track=\"click\" data-track-label=\"image\" data-track-action=\"view figure\" href=\"https:\/\/www.nature.com\/articles\/s41467-025-65528-y\/figures\/1\" rel=\"nofollow noopener\" target=\"_blank\"><img decoding=\"async\" aria-describedby=\"Fig1\" src=\"https:\/\/www.newsbeep.com\/ca\/wp-content\/uploads\/2025\/10\/41467_2025_65528_Fig1_HTML.png\" alt=\"figure 1\" loading=\"lazy\" width=\"685\" height=\"388\"\/><\/a><\/p>\n<p>a False-colored scanning electron microscope (SEM) image of the qubit circuit, galvanically coupled to the readout resonator. The device consists of a 20\u2009nm thick single layer of grAl. The colored regions (ocher &amp; violet) illustrate the 10% mismatched areas of the two flux loops in the gradiometric design<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 48\" title=\"Gusenkova, D. et al. Operating in a deep underground facility improves the locking of gradiometric fluxonium qubits at the sweet spots. Appl. Phys. Lett. 120, &#010;                  https:\/\/doi.org\/10.1063\/5.0075909&#010;                  &#010;                 (2022).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR48\" id=\"ref-link-section-d54651764e1644\" rel=\"nofollow noopener\" target=\"_blank\">48<\/a>, which result in an effective flux bias \u03a6ext in perpendicular magnetic field B\u22a5 (cf. Eq. (<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"equation anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Equ2\" rel=\"nofollow noopener\" target=\"_blank\">2<\/a>)). Inset: zoom-in on the \u00a0~20\u2009nm wide grAl nanojunction of the qubit (cf.\u00a0ref.\u00a0<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 46\" title=\"Rieger, D. et al. Granular aluminium nanojunction fluxonium qubit. Nat. Mater. 22, 194 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR46\" id=\"ref-link-section-d54651764e1658\" rel=\"nofollow noopener\" target=\"_blank\">46<\/a>). b Circuit schematic for the gradiometric qubit depicted in a: the nanojunction (red) is shunted by an interdigitated capacitor and two flux loops (ocher &amp; violet) with inductances L1\u2009+\u2009Ls and L3, respectively. The inductance shared between the loops is L2. The qubit is inductively coupled via Ls to the readout resonator (inductance Lr, capacitance Cr) for which we measure the single-port reflection coefficient S11. c Two-tone (TT) spectroscopy at the half flux sweet spot \u03a6ext\u2009=\u2009\u03a60\/2 in B\u2225\u2009=\u20090\u2009T. d Increase of the sweet spot qubit frequency in magnetic field up to 1.2\u2009T. Inset: TT-spectroscopy in B\u2225\u2009=\u20091.2\u2009T. e Qubit spectrum: ground to excited (fge in dark blue markers) and ground to second-excited (fgf in light blue markers) state transitions extracted from TT-spectroscopy. From a fit (black line) to the fluxonium Hamiltonian (Eq. (<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"equation anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Equ1\" rel=\"nofollow noopener\" target=\"_blank\">1<\/a>)), we obtain EJ\/h\u2009=\u200932.2\u2009GHz (i.e., critical current Ic\u2009=\u200964.9\u2009nA), Ec\/h\u2009=\u200914.1\u2009GHz (C\u2009=\u20091.37\u2009fF) and EL\/h\u2009=\u20090.454\u2009GHz (Lq\u2009=\u2009360\u2009nH). f Suppression of the grAl superconducting gap \u0394 in magnetic field. The red and orange markers, corresponding to the qubit nanojunction and inductor superconducting gaps (\\({\\Delta }_{{E}_{{{\\rm{J}}}}}\\), \\({\\Delta }_{{L}_{{{\\rm{q}}}}}\\)), are obtained from fitted EJ and EL values (cf. e) at each magnetic field. The capacitance C is fixed to the fit value obtained in B\u2225\u2009=\u20090\u2009T. The green markers are obtained from the shift of the readout resonator frequency fr(B\u2225). The black lines show fits to the field dependence of the superconducting gap, indicating a 40% higher critical field for the nanojunction.<\/p>\n<p>From two-tone (TT) spectroscopy at half flux bias \u03a6\u2009=\u2009\u03a60\/2 shown in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1c<\/a>, we determine a qubit frequency of fq(\u03a60\/2)\u2009=\u20092.365\u2009GHz in zero field, B\u2225\u2009=\u20090. Remarkably, as shown in Fig. <a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1d<\/a>, tracking the sweet spot qubit frequency in magnetic field reveals only a 1% increase (32\u2009MHz) up to 1.2\u2009T, illustrating the compatibility of the gradiometric gralmonium qubit with high magnetic fields. The spectroscopy data in 1.2\u2009T is blurred compared to zero field due to low-frequency flux noise, likely from vibrations of the sample holder inside the vector magnet (cf. Supplementary <a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">I<\/a>). Figure\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1e<\/a> shows the gralmonium spectrum up to 13\u2009GHz, extracted from TT spectroscopy. A joint fit of the qubit transitions \\(\\left\\vert \\,{\\mbox{g}}\\,\\right\\rangle \\to \\left\\vert \\,{\\mbox{e}}\\,\\right\\rangle\\) and \\(\\left\\vert \\,{\\mbox{g}}\\,\\right\\rangle \\to \\left\\vert \\,{\\mbox{f}}\\,\\right\\rangle\\) to a numerical diagonalization of Eq. (<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"equation anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Equ1\" rel=\"nofollow noopener\" target=\"_blank\">1<\/a>) yields typical fluxonium parameters: EJ\/h\u2009=\u200932.2\u2009GHz, Ec\/h\u2009=\u200914.1\u2009GHz and EL\/h\u2009=\u20090.454\u2009GHz.<\/p>\n<p>To assess the effect of the magnetic field on the fluxonium parameters, we measure the qubit ground to excited transition frequency fge near the half- and zeroflux sweet spots at each B\u2225, using TT spectroscopy (similar to Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1c<\/a>). We fit fge to Eq.(<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"equation anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Equ1\" rel=\"nofollow noopener\" target=\"_blank\">1<\/a>) using the field independent capacitance C\u2009=\u20091.37\u2009fF obtained in zero field. From the fitted parameters, using EJ\u2009\u221d\u2009\u0394(B\u2225) and Lkin\u2009\u221d\u20091\/\u0394(B\u2225), we extract the magnetic field suppression of the superconducting gap in the superinductor (\\(\\delta {\\Delta }_{{L}_{{{\\rm{q}}}}}\\)) and nanojunction (\\(\\delta {\\Delta }_{{E}_{{{\\rm{J}}}}}\\)), as shown in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig1\" rel=\"nofollow noopener\" target=\"_blank\">1f<\/a>. The suppression of the resonator superconducting gap (\\(\\delta {\\Delta }_{{L}_{{{\\rm{r}}}}}\\)) is independently obtained by fitting the resonance frequency shift \\({f}_{{{\\rm{r}}}}\\propto 1\/\\sqrt{{L}_{{{\\rm{kin}}}}}\\). Interestingly, the nanojunction has an even higher field resilience than the grAl resonator and superinductor. We fit the relative gap suppression to \\(\\sqrt{1-{({B}_{\\parallel }\/{B}_{{{\\rm{c}}}})}^{2}}\\)<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 49\" title=\"Douglass, D. H. Magnetic field dependence of the superconducting energy gap. Phys. Rev. Lett. 6, 346 (1961).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR49\" id=\"ref-link-section-d54651764e2342\" rel=\"nofollow noopener\" target=\"_blank\">49<\/a> and obtain a critical field \\({B}_{{{\\rm{c}}}}^{{E}_{{{\\rm{J}}}}}=6.8\\,{{\\rm{T}}}\\) for the nanojunction and \\({B}_{{{\\rm{c}}}}^{{{\\rm{L}}}}=4.9\\,{{\\rm{T}}}\\) for the resonator and qubit inductance. The fact that \\({B}_{{{\\rm{c}}}}^{{E}_{{{\\rm{J}}}}} &gt; {B}_{{{\\rm{c}}}}^{{{\\rm{L}}}}\\) indicates that possible Fraunhofer interference in the nanojunction plays a minor role. The higher critical field of the nanojunction is not understood and could be due to its reduced dimensions, similar to ref. <a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 50\" title=\"Deshpande, A. et al. Tuning the superconducting dome in granular aluminum thin films. J. Appl. Phys. 137, &#010;                  https:\/\/doi.org\/10.1063\/5.0250146&#010;                  &#010;                 (2025).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR50\" id=\"ref-link-section-d54651764e2519\" rel=\"nofollow noopener\" target=\"_blank\">50<\/a>.<\/p>\n<p>We quantify the quantum coherence of the gralmonium in field by performing time-domain measurements at the half flux sweet spot, as summarized in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2<\/a>. Remarkably, the energy relaxation time T1 and Hahn echo coherence time T2E remain robust in fields up to 1.2\u2009T, the upper limit of our vector magnet (cf. Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2a<\/a>). The Ramsey coherence time T2R decreases from a maximum of T2R\u2009=\u20091.5\u2009\u03bcs to T2R\u2009=\u20090.7\u2009\u03bcs in fields above 1\u2009T. We attribute this to an increase of low frequency flux noise, which stems from global flux variations introduced by vibrations and activated vortices in the vector magnet<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 51\" title=\"Schwarz, T. et al. Low-noise nano superconducting quantum interference device operating in tesla magnetic fields. ACS Nano 7, 844 (2013).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR51\" id=\"ref-link-section-d54651764e2553\" rel=\"nofollow noopener\" target=\"_blank\">51<\/a>, or from local flux noise, possibly from spins clusters<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 38\" title=\"Rower, D. A. et al. Evolution of 1\/f flux noise in superconducting qubits with weak magnetic fields. Phys. Rev. Lett. 130, 220602 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR38\" id=\"ref-link-section-d54651764e2558\" rel=\"nofollow noopener\" target=\"_blank\">38<\/a>.<\/p>\n<p>Fig. 2: Qubit coherence in magnetic field: signatures of environmental spin polarization.<a class=\"c-article-section__figure-link\" data-test=\"img-link\" data-track=\"click\" data-track-label=\"image\" data-track-action=\"view figure\" href=\"https:\/\/www.nature.com\/articles\/s41467-025-65528-y\/figures\/2\" rel=\"nofollow noopener\" target=\"_blank\"><img decoding=\"async\" aria-describedby=\"Fig2\" src=\"https:\/\/www.newsbeep.com\/ca\/wp-content\/uploads\/2025\/10\/41467_2025_65528_Fig2_HTML.png\" alt=\"figure 2\" loading=\"lazy\" width=\"685\" height=\"388\"\/><\/a><\/p>\n<p>a Energy relaxation time T1, Ramsey and echo coherence time, T2R and T2E respectively, of the gradiometric gralmonium in magnetic field up to 1\u2009T. b, c Ramsey fringes measured in B\u2225\u2009=\u20090\u2009T and B\u2225\u2009=\u20091\u2009T, respectively. A two-frequency fit (black line) indicates a similar beating pattern (dotted envelope) for both magnetic fields. d Energy relaxation T1 up to 120\u2009mT: similarly to observations on resonators<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 39\" title=\"Borisov, K. et al. Superconducting granular aluminum resonators resilient to magnetic fields up to 1 Tesla. Appl. Phys. Lett. 117, &#010;                  https:\/\/doi.org\/10.1063\/5.0018012&#010;                  &#010;                 (2020).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR39\" id=\"ref-link-section-d54651764e2611\" rel=\"nofollow noopener\" target=\"_blank\">39<\/a>&#8211;<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 41\" title=\"Kroll, J. G. et al. Magnetic-field-resilient superconducting coplanar-waveguide resonators for hybrid circuit quantum electrodynamics experiments. Phys. Rev. Appl. 11, 064053 (2019).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR41\" id=\"ref-link-section-d54651764e2615\" rel=\"nofollow noopener\" target=\"_blank\">41<\/a>, the drop in T1 suggests coupling to the electron spin resonance (ESR) of paramagnetic impurities of unknown origin. Inset: The fields BESR\u2009=\u2009hfq\/g\u03bcB at which the ESR matches different qubit frequencies in different cooldowns, correspond to the expectation for a spin s\u2009=\u20091\/2 ensemble with gyromagnetic factor g\u2009=\u20092 (black line). Note that we use the same device for which the qubit frequency changes between cooldowns (cf. ref. <a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 46\" title=\"Rieger, D. et al. Granular aluminium nanojunction fluxonium qubit. Nat. Mater. 22, 194 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR46\" id=\"ref-link-section-d54651764e2647\" rel=\"nofollow noopener\" target=\"_blank\">46<\/a>). e Dephasing times T\u03c6R, T\u03c6E remain unaffected by the ESR. f Flux noise echo dephasing rate \\({\\Gamma }_{\\varphi \\,{\\mbox{E}}\\,}^{\\Phi }\\) in the vicinity of the sweet spot for three in-plane magnetic fields. Dashed lines show fits to Eq. (<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"equation anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Equ3\" rel=\"nofollow noopener\" target=\"_blank\">3<\/a>). g Flux noise amplitude \\(\\sqrt{{A}_{\\Phi }}\\) in magnetic field with fit to Eq. (<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"equation anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Equ4\" rel=\"nofollow noopener\" target=\"_blank\">4<\/a>), corresponding to a spin freezing with a spin temperature of TS\u2009=\u200985\u2009mK. In all panels, the error bars represent the standard deviation obtained from successive measurements.<\/p>\n<p>The grAl nanojunction exhibits critical current fluctuations, as evidenced by a 0.5\u2009MHz toggling of the qubit frequency and a corresponding beating pattern in Ramsey fringes at zero field (cf. Fig. <a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2b<\/a>). As demonstrated in ref. <a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 46\" title=\"Rieger, D. et al. Granular aluminium nanojunction fluxonium qubit. Nat. Mater. 22, 194 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR46\" id=\"ref-link-section-d54651764e2778\" rel=\"nofollow noopener\" target=\"_blank\">46<\/a>, these fluctuations are inconsistent with transverse coupling to a fixed frequency TLS, but originate from fluctuations of the nanojunction energy, potentially arising from structural defects, charge noise, or paramagnetic impurities. This issue is also relevant for standard Al\/AlOx\/Al tunnel JJs<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 30\" title=\"Nugroho, C. D., Orlyanchik, V. &amp; Van Harlingen, D. J. Low frequency resistance and critical current fluctuations in Al-based Josephson junctions. Appl. Phys. Lett. 102, 142602 (2013).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR30\" id=\"ref-link-section-d54651764e2786\" rel=\"nofollow noopener\" target=\"_blank\">30<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 52\" title=\"Van Harlingen, D. J. et al. Decoherence in Josephson-junction qubits due to critical-current fluctuations. Phys. Rev. B 70, 064517 (2004).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR52\" id=\"ref-link-section-d54651764e2789\" rel=\"nofollow noopener\" target=\"_blank\">52<\/a>. We leverage the gradiometric gralmonium\u2019s field resilience to test the magnetic susceptibility of critical current noise, showing in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2c<\/a> that a 1\u2009T in-plane magnetic field does not suppress the discrete fluctuations of the Josephson energy. This observation excludes magnetically susceptible sources, such as a local spin environment, as the origin of these fluctuations. Further experiments, such as electric field bias or mechanical strain on the substrate<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 32\" title=\"M&#xFC;ller, C., Cole, J. H. &amp; Lisenfeld, J. Towards understanding two-level-systems in amorphous solids: insights from quantum circuits. Rep. Prog. Phys. 82, 124501 (2019).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR32\" id=\"ref-link-section-d54651764e2797\" rel=\"nofollow noopener\" target=\"_blank\">32<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 53\" title=\"Kristen, M. et al. Giant two-level systems in a granular superconductor. Phys. Rev. Lett. 132, 217002 (2024).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR53\" id=\"ref-link-section-d54651764e2800\" rel=\"nofollow noopener\" target=\"_blank\">53<\/a> or spin-locking TLS spectroscopy<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 54\" title=\"Abdurakhimov, L. V. et al. Identification of different types of high-frequency defects in superconducting qubits. PRX Quantum 3, 040332 (2022).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR54\" id=\"ref-link-section-d54651764e2804\" rel=\"nofollow noopener\" target=\"_blank\">54<\/a>, are required to identify their cause.<\/p>\n<p>We observe a dip in the energy relaxation time at the magnetic field where the electron spin resonance (ESR) matches the qubit frequency hf\u2009=\u2009g\u03bcBB (cf. Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2d<\/a>). This ESR resonance does not impact the dephasing times T\u03c6R, T\u03c6E (cf. Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2e<\/a>), as expected in the limit of a coupling strength much smaller than the qubit linewidth<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 55\" title=\"Spiecker, M., Pavlov, A. I., Shnirman, A. &amp; Pop, I. M. Solomon equations for qubit and two-level systems: Insights into non-Poissonian quantum jumps. Phys. Rev. A 109, 052218 (2024).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR55\" id=\"ref-link-section-d54651764e2840\" rel=\"nofollow noopener\" target=\"_blank\">55<\/a>. By exploiting \u0394EJ\u2009~\u2009GHz changes in the nanojunction energy after thermal cycling, we change the qubit frequency of the same device, allowing measurements of the ESR-resonant field BESR across multiple qubit frequencies at the half flux sweet spot (inset of Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2d<\/a>). The linear trend of the extracted magnetic fields BESR aligns with the prediction for a g\u2009=\u20092 spin s\u2009=\u20091\/2 ensemble, identifying a paramagnetic spin ensemble coupled to our qubit.<\/p>\n<p>Figure\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2f<\/a> illustrates the flux dependence of the Hahn echo flux noise dephasing rate, \\({\\Gamma }_{\\varphi \\,{\\mbox{E}}\\,}^{\\Phi }\\), near the sweet spot for three in-plane magnetic fields (B\u2225\u2009=\u20090, B\u2225\u2009=\u20090.3\u2009T, B\u2225\u2009=\u20090.6\u2009T). Away from the sweet spot, we observe a Gaussian contribution in the Hahn echo decay curve, consistent with commonly observed 1\/f flux noise<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" title=\"Braum&#xFC;ller, J. et al. Characterizing and optimizing qubit coherence based on SQUID geometry. Phys. Rev. Appl. 13, 054079 (2020).\" href=\"#ref-CR27\" id=\"ref-link-section-d54651764e2930\">27<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" title=\"Stern, M. et al. Flux qubits with long coherence times for hybrid quantum circuits. Phys. Rev. Lett. 113, 123601 (2014).\" href=\"#ref-CR28\" id=\"ref-link-section-d54651764e2930_1\">28<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" title=\"Yoshihara, F., Harrabi, K., Niskanen, A. O., Nakamura, Y. &amp; Tsai, J. S. Decoherence of flux qubits due to 1\/f flux noise. Phys. Rev. Lett. 97, 167001 (2006).\" href=\"#ref-CR29\" id=\"ref-link-section-d54651764e2930_2\">29<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" title=\"Nugroho, C. D., Orlyanchik, V. &amp; Van Harlingen, D. J. Low frequency resistance and critical current fluctuations in Al-based Josephson junctions. Appl. Phys. Lett. 102, 142602 (2013).\" href=\"#ref-CR30\" id=\"ref-link-section-d54651764e2930_3\">30<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 31\" title=\"Yan, F. et al. The flux qubit revisited to enhance coherence and reproducibility. Nat. Commun. 7, 1 (2016).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR31\" id=\"ref-link-section-d54651764e2933\" rel=\"nofollow noopener\" target=\"_blank\">31<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 38\" title=\"Rower, D. A. et al. Evolution of 1\/f flux noise in superconducting qubits with weak magnetic fields. Phys. Rev. Lett. 130, 220602 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR38\" id=\"ref-link-section-d54651764e2936\" rel=\"nofollow noopener\" target=\"_blank\">38<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 56\" title=\"Schriefl, J., Makhlin, Y., Shnirman, A. &amp; Sch&#xF6;n, G. Decoherence from ensembles of two-level fluctuators. New J. Phys. 8, 1 (2006).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR56\" id=\"ref-link-section-d54651764e2939\" rel=\"nofollow noopener\" target=\"_blank\">56<\/a>. We extract \\({\\Gamma }_{\\varphi \\,{\\mbox{E}}\\,}^{\\Phi }\\) from the flux-dependent Gaussian envelope \\({e}^{-{({\\Gamma }_{\\varphi {\\mbox{E}}}^{\\Phi }t)}^{2}}\\), on top of a purely exponential decay \\({e}^{-({\\Gamma }_{1}\/2+{\\Gamma }_{\\varphi {\\mbox{E}}}^{{{\\rm{const}}}})t}\\), extracted at \u03a6\u2009=\u2009\u03a60\/2. The flux-independent term \\({\\Gamma }_{\\varphi \\,{\\mbox{E}}}^{{\\mbox{const}}\\,}\\) may originate from critical current noise or photon shot noise; in the latter case, the residual photon number is \\(\\bar{n}=0.27\\), corresponding to an effective temperature of 150\u2009mK, in agreement with the qubit temperature (cf. Supplementary <a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">I<\/a>). Interestingly, the flux dependence \\({\\Gamma }_{\\varphi \\,{\\mbox{E}}}^{\\Phi }({\\Phi }_{{{\\rm{ext}}}})\\) weakens as the magnetic field B\u2225 increases (cf. Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2f<\/a>), reminiscent of earlier observations in flux qubits at lower field<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 38\" title=\"Rower, D. A. et al. Evolution of 1\/f flux noise in superconducting qubits with weak magnetic fields. Phys. Rev. Lett. 130, 220602 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR38\" id=\"ref-link-section-d54651764e3302\" rel=\"nofollow noopener\" target=\"_blank\">38<\/a>. We fit the flux noise amplitude \\(\\sqrt{{A}_{\\Phi }}\\) for a S\u03a6(\u03c9)\u2009=\u2009A\u03a6\/\u03c9 power spectral density using<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 29\" title=\"Yoshihara, F., Harrabi, K., Niskanen, A. O., Nakamura, Y. &amp; Tsai, J. S. Decoherence of flux qubits due to 1\/f flux noise. Phys. Rev. Lett. 97, 167001 (2006).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR29\" id=\"ref-link-section-d54651764e3356\" rel=\"nofollow noopener\" target=\"_blank\">29<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 56\" title=\"Schriefl, J., Makhlin, Y., Shnirman, A. &amp; Sch&#xF6;n, G. Decoherence from ensembles of two-level fluctuators. New J. Phys. 8, 1 (2006).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR56\" id=\"ref-link-section-d54651764e3359\" rel=\"nofollow noopener\" target=\"_blank\">56<\/a>.<\/p>\n<p>$${\\Gamma }_{\\varphi \\,{\\mbox{E}}\\,}^{\\Phi }=\\sqrt{{A}_{\\Phi }\\ln 2}\\left\\vert \\frac{\\partial \\omega }{\\partial {\\Phi }_{{{\\rm{ext}}}}}\\right\\vert \\,.$$<\/p>\n<p>\n                    (3)\n                <\/p>\n<p>With increasing B\u2225, we observe a decrease of \\(\\sqrt{{A}_{\\Phi }}\\) by a factor of \u00a0~2, reported in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2g<\/a>, which holds across different qubit frequencies in several cooldowns (cf. Supplementary\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">III<\/a>). However, for B\u2225\u2009\u2273\u20091\u2009T, \\(\\sqrt{{A}_{\\Phi }}\\) increases, suggesting the onset of a competing mechanism, likely due to vortex dynamics in the magnet wires.<\/p>\n<p>We model the flux noise as the sum of a large number of magnetic two-level fluctuators, consistent with the commonly accepted spin-based origin of flux noise<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" title=\"Lanting, T. et al. Geometrical dependence of the low-frequency noise in superconducting flux qubits. Phys. Rev. B 79, 060509 (2009).\" href=\"#ref-CR57\" id=\"ref-link-section-d54651764e3565\">57<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" title=\"Quintana, C. M. et al. Observation of classical-quantum crossover of 1\/f flux noise and its paramagnetic temperature dependence. Phys. Rev. Lett. 118, 057702 (2017).\" href=\"#ref-CR58\" id=\"ref-link-section-d54651764e3565_1\">58<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 59\" title=\"Gao, R. et al. The effects of disorder in superconducting materials on qubit coherence. Nat. Commun. 16, 1 (2025).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR59\" id=\"ref-link-section-d54651764e3568\" rel=\"nofollow noopener\" target=\"_blank\">59<\/a>. Each of them constitutes a source of asymmetric random telegraphic noise, with a Lorentzian power spectrum \\(S(\\omega )\\propto {({\\Gamma }_{1}\/{\\Gamma }_{\\uparrow }+{\\Gamma }_{1}\/{\\Gamma }_{\\downarrow })}^{-1}\\cdot {\\Gamma }_{1}\/({\\Gamma }_{1}^{2}+{\\omega }^{2})\\), where \u03931\u2009=\u2009\u0393\u2191\u2009+\u2009\u0393\u2193 are the excitation and relaxation rates of the fluctuator, respectively<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 60\" title=\"Kogan, Sh. Electronic noise and fluctuations in solids (Cambridge University Press, 1996).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR60\" id=\"ref-link-section-d54651764e3766\" rel=\"nofollow noopener\" target=\"_blank\">60<\/a>. In the limit of identical fluctuators, S(\u03c9) remains Lorentzian, while for fluctuators with 1\/\u03931 uniformly distributed, S(\u03c9)\u2009\u221d\u20091\/\u03c9<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 56\" title=\"Schriefl, J., Makhlin, Y., Shnirman, A. &amp; Sch&#xF6;n, G. Decoherence from ensembles of two-level fluctuators. New J. Phys. 8, 1 (2006).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR56\" id=\"ref-link-section-d54651764e3787\" rel=\"nofollow noopener\" target=\"_blank\">56<\/a>. However, for any distribution, the amplitude of the power spectrum is \\({A}_{\\Phi }\\propto {({\\Gamma }_{1}\/{\\Gamma }_{\\uparrow }+{\\Gamma }_{1}\/{\\Gamma }_{\\downarrow })}^{-1}\\), which becomes (cf. Supplementary <a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">III<\/a>).<\/p>\n<p>$${A}_{\\Phi }\\propto 1\/{\\cosh }^{2}\\left(\\frac{{\\mu }_{{{\\rm{B}}}}B}{{k}_{{{\\rm{B}}}}{T}_{{{\\rm{S}}}}}\\right)\\,.$$<\/p>\n<p>\n                    (4)\n                <\/p>\n<p>Here, 2\u03bcBB is the energy of g\u2009=\u20092,\u00a0s\u2009=\u20091\/2 paramagnetic impurities and \u03bcB, kB and TS are the Bohr magneton, the Boltzmann constant and the spin bath temperature, respectively. A fit with TS\u2009=\u200985\u2009mK aligns with the measured flux noise amplitude (black line in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2g<\/a>) up to 1\u2009T. This suggests the freezing of g\u2009=\u20092 paramagnetic impurities responsible for the reduction of flux noise, presumably the same spin environment that causes the T1 dip (cf. Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2d<\/a>).<\/p>\n<p>In Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig3\" rel=\"nofollow noopener\" target=\"_blank\">3<\/a>, we leverage the field resilience of the gralmonium to probe the magnetic susceptibility of a recently discovered TLS bath coupled to superconducting qubits<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 34\" title=\"Spiecker, M. et al. Two-level system hyperpolarization using a quantum Szilard engine. Nat. Phys. 19, 1320 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR34\" id=\"ref-link-section-d54651764e4080\" rel=\"nofollow noopener\" target=\"_blank\">34<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 47\" title=\"Zhuang, Z. T. et al. Non-Markovian relaxation spectroscopy of fluxonium qubits. Preprint at &#010;                  https:\/\/doi.org\/10.48550\/arXiv.2503.16381&#010;                  &#010;                 (2025).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR47\" id=\"ref-link-section-d54651764e4083\" rel=\"nofollow noopener\" target=\"_blank\">47<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 55\" title=\"Spiecker, M., Pavlov, A. I., Shnirman, A. &amp; Pop, I. M. Solomon equations for qubit and two-level systems: Insights into non-Poissonian quantum jumps. Phys. Rev. A 109, 052218 (2024).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR55\" id=\"ref-link-section-d54651764e4086\" rel=\"nofollow noopener\" target=\"_blank\">55<\/a>. These TLSs have been shown to induce non-Markovian qubit dynamics, and their long lifetime, exceeding 1\/\u0393TLS\u2009\u226550\u2009ms, makes a spin-based origin plausible. Following ref. <a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 34\" title=\"Spiecker, M. et al. Two-level system hyperpolarization using a quantum Szilard engine. Nat. Phys. 19, 1320 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR34\" id=\"ref-link-section-d54651764e4092\" rel=\"nofollow noopener\" target=\"_blank\">34<\/a>, by repeatedly preparing the qubit in either \\(\\left\\vert \\,{\\mbox{g}}\\,\\right\\rangle\\) or \\(\\left\\vert \\,{\\mbox{e}}\\,\\right\\rangle\\) using fast feedback over N\u2009=\u2009104 iterations, the TLS ensemble hyperpolarizes via its cross-relaxation to the qubit. After this polarization sequence, the qubit is initialized in either \\(\\left\\vert \\,{\\mbox{g}}\\,\\right\\rangle\\) or \\(\\left\\vert \\,{\\mbox{e}}\\,\\right\\rangle\\), and its population is monitored using stroboscopic quantum jump measurements. Figure\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig3\" rel=\"nofollow noopener\" target=\"_blank\">3b<\/a> shows the distinct signatures of a hyperpolarized long-lived TLS ensemble coupled to the gralmonium: regardless of the qubit\u2019s initial state, it relaxes to the TLS ensemble population on a T1 timescale, while the TLS ensemble itself decays to thermal equilibrium on milliseconds timescale. By modeling the qubit coupled to a ladder of 102 TLSs<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 34\" title=\"Spiecker, M. et al. Two-level system hyperpolarization using a quantum Szilard engine. Nat. Phys. 19, 1320 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR34\" id=\"ref-link-section-d54651764e4224\" rel=\"nofollow noopener\" target=\"_blank\">34<\/a>, we extract a gralmonium relaxation \u03931\u2009=\u20091\/5.4\u2009\u03bcs, of which TLS cross-relaxation accounts for \\({\\sum }_{k}{\\Gamma }_{\\,{\\mbox{qt}}\\,}^{k}=1\/22\\,\\mu {{\\rm{s}}}\\).<\/p>\n<p>Fig. 3: Magnetic susceptibility of long-lived two-level-systems (TLSs) in high field.<a class=\"c-article-section__figure-link\" data-test=\"img-link\" data-track=\"click\" data-track-label=\"image\" data-track-action=\"view figure\" href=\"https:\/\/www.nature.com\/articles\/s41467-025-65528-y\/figures\/3\" rel=\"nofollow noopener\" target=\"_blank\"><img decoding=\"async\" aria-describedby=\"Fig3\" src=\"https:\/\/www.newsbeep.com\/ca\/wp-content\/uploads\/2025\/10\/41467_2025_65528_Fig3_HTML.png\" alt=\"figure 3\" loading=\"lazy\" width=\"685\" height=\"194\"\/><\/a><\/p>\n<p>a Sketch of the qubit preparation sequence used in (b\u2013d). The repeated (N\u2009=\u2009104) active reset of the qubit state in \\(\\left\\vert \\,{\\mbox{g}}\\,\\right\\rangle\\) or \\(\\left\\vert \\,{\\mbox{e}}\\,\\right\\rangle\\) (blue and red traces in all panels, respectively) results in the hyperpolarization of environmental, long-lived TLS<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 34\" title=\"Spiecker, M. et al. Two-level system hyperpolarization using a quantum Szilard engine. Nat. Phys. 19, 1320 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR34\" id=\"ref-link-section-d54651764e4385\" rel=\"nofollow noopener\" target=\"_blank\">34<\/a>. The last step of the preparation sequence consists in a qubit initialization in \\(\\left\\vert \\,{\\mbox{g}}\\,\\right\\rangle\\) or \\(\\left\\vert \\,{\\mbox{e}}\\,\\right\\rangle\\). We use a 540\u2009ns rectangular readout pulse and a 32\u2009ns Gaussian \u03c0-pulse. b Qubit population relaxation after the preparation sequence for different magnetic fields B\u2225. We fit the data (semi-transparent) to the theoretical model<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 34\" title=\"Spiecker, M. et al. Two-level system hyperpolarization using a quantum Szilard engine. Nat. Phys. 19, 1320 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR34\" id=\"ref-link-section-d54651764e4456\" rel=\"nofollow noopener\" target=\"_blank\">34<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 55\" title=\"Spiecker, M., Pavlov, A. I., Shnirman, A. &amp; Pop, I. M. Solomon equations for qubit and two-level systems: Insights into non-Poissonian quantum jumps. Phys. Rev. A 109, 052218 (2024).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR55\" id=\"ref-link-section-d54651764e4459\" rel=\"nofollow noopener\" target=\"_blank\">55<\/a> (opaque). For reference, the black dashed lines show an exponential decay with the qubit energy relaxation rate \u03931. In zero field, we reproduce the signatures of TLS hyperpolarization recently observed in other superconducting qubits<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 34\" title=\"Spiecker, M. et al. Two-level system hyperpolarization using a quantum Szilard engine. Nat. Phys. 19, 1320 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR34\" id=\"ref-link-section-d54651764e4465\" rel=\"nofollow noopener\" target=\"_blank\">34<\/a>,<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 35\" title=\"Odeh, M. et al. Non-Markovian dynamics of a superconducting qubit in a phononic bandgap. Nat. Phys. &#010;                  https:\/\/doi.org\/10.1038\/s41567-024-02740-5&#010;                  &#010;                 (2025).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR35\" id=\"ref-link-section-d54651764e4468\" rel=\"nofollow noopener\" target=\"_blank\">35<\/a>, i.e., undershoot (blue) and overshoot (red) compared to the single exponential decay. c At the ESR resonance field BESR, the hyperpolarization signatures are suppressed due to energy relaxation of the qubit into the paramagnetic ensemble. d The signatures of TLS hyperpolarization on qubit relaxation in magnetic fields exceeding 1\u2009T are comparable to zero field, indicating a very low susceptibility of the long-lived TLSs to magnetic field.<\/p>\n<p>In magnetic field, the signatures of TLS hyperpolarization remain visible, as illustrated in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig3\" rel=\"nofollow noopener\" target=\"_blank\">3c, d<\/a>. The fact that the hyperpolarization in B\u2225\u2009=\u20091.2\u2009T is comparable to zero field indicates that the TLS bath is not magnetically susceptible, ruling out origins, such as electronic spins. Remaining non-magnetically-susceptible microscopic origins include subgap states, possibly trapped quasiparticles<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 61\" title=\"de Graaf, S. E. et al. Two-level systems in superconducting quantum devices due to trapped quasiparticles. Sci. Adv. 6, &#010;                  https:\/\/doi.org\/10.1126\/sciadv.abc5055&#010;                  &#010;                 (2020).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR61\" id=\"ref-link-section-d54651764e4501\" rel=\"nofollow noopener\" target=\"_blank\">61<\/a>. As shown in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig3\" rel=\"nofollow noopener\" target=\"_blank\">3c<\/a>, at B\u2009\u2248\u2009BESR, where T1 is suppressed by a factor of 7 (cf. Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2d<\/a>), the TLS hyperpolarization is less pronounced. Therefore, we are still able to hyperpolarize the long-lived TLSs, but not the paramagnetic spins. This indicates that the spin ensemble is large enough or sufficiently coupled to the environment that it embodies a Markovian bath. In contrast, the long-lived TLS environment appears to be uncoupled to the spin ensemble, as evidenced by the fit in Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#Fig3\" rel=\"nofollow noopener\" target=\"_blank\">3c<\/a> with a practically unchanged cross-relaxation rate of \\({\\sum }_{k}{\\Gamma }_{\\,{\\mbox{qt}}\\,}^{k}=1\/33\\,\\mu {{\\rm{s}}}\\).<\/p>\n<p>In conclusion, we have introduced a field-resilient superconducting qubit\u2014the gradiometric gralmonium\u2014that operates robustly in Tesla magnetic fields. By incorporating a grAl nanojunction, the gralmonium maintains spectral stability and coherence in high magnetic fields, circumventing the Fraunhofer interference typically observed in JJ-based superconducting circuits. We reveal distinct properties of spin environments coupled to the gralmonium by addressing their magnetic field susceptibility. Using ESR, we characterize a paramagnetic spin-1\/2 ensemble that couples transversely to the qubit, demonstrating the gralmonium\u2019s potential as a probe for spin dynamics. We confirm the long-standing hypothesis of the freeze-out of fast flux noise in high fields, consistent with a spin s\u2009=\u2009\u00a01\/2, g\u2009=\u20092 paramagnetic origin. The operation of the gralmonium in magnetic field also allowed us to disprove the electron-spin hypothesis for the long-lived two-level system (TLS) environment responsible for non-Markovian qubit dynamics.<\/p>\n<p>Future work should address flux noise suppression and spectral noise analysis, and should validate the correlation between flux noise and the spin-1\/2 ensemble in order to gain insights into its microscopic origin. Most importantly, the gralmonium\u2019s resilience to magnetic fields offers a promising path forward in hybrid quantum architectures, facilitating seamless integration with magnetic-field-sensitive systems, such as spins<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 62\" title=\"G&#xFC;nzler, S. et al. Kinetic inductance coupling for circuit QED with spins. Phys. Rev. B 112, 115424 (2025).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-65528-y#ref-CR62\" id=\"ref-link-section-d54651764e4611\" rel=\"nofollow noopener\" target=\"_blank\">62<\/a>, magnons, or topological materials.<\/p>\n","protected":false},"excerpt":{"rendered":"In Fig.\u00a01 we present the field resilient gralmonium qubit, fabricated from a single layer of grAl (cf. Fig.\u00a01a),&hellip;\n","protected":false},"author":2,"featured_media":249192,"comment_status":"","ping_status":"","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[24],"tags":[49,48,1099,1100,314,3230,8269,66,16968,3884],"class_list":{"0":"post-249191","1":"post","2":"type-post","3":"status-publish","4":"format-standard","5":"has-post-thumbnail","7":"category-physics","8":"tag-ca","9":"tag-canada","10":"tag-humanities-and-social-sciences","11":"tag-multidisciplinary","12":"tag-physics","13":"tag-quantum-information","14":"tag-qubits","15":"tag-science","16":"tag-superconducting-devices","17":"tag-superconducting-properties-and-materials"},"_links":{"self":[{"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/posts\/249191","targetHints":{"allow":["GET"]}}],"collection":[{"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/posts"}],"about":[{"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/users\/2"}],"replies":[{"embeddable":true,"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/comments?post=249191"}],"version-history":[{"count":0,"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/posts\/249191\/revisions"}],"wp:featuredmedia":[{"embeddable":true,"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/media\/249192"}],"wp:attachment":[{"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/media?parent=249191"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/categories?post=249191"},{"taxonomy":"post_tag","embeddable":true,"href":"https:\/\/www.newsbeep.com\/ca\/wp-json\/wp\/v2\/tags?post=249191"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}