Degen, C. L., Reinhard, F. & Cappellaro, P. Quantum sensing. Rev. Mod. Phys. 89, 035002 (2017).
Casola, F., van der Sar, T. & Yacoby, A. Probing condensed matter physics with magnetometry based on nitrogen-vacancy centres in diamond. Nat. Rev. Mater. 3, 17088 (2018).
Rovny, J. et al. Nanoscale diamond quantum sensors for many-body physics. Nat. Rev. Phys. 6, 753–768 (2024).
Aslam, N. et al. Quantum sensors for biomedical applications. Nat. Rev. Phys. 5, 157–169 (2023).
Crawford, S. E. et al. Quantum sensing for energy applications: review and perspective. Adv. Quantum Technol. 4, 2100049 (2021).
Ye, J. & Zoller, P. Essay: quantum sensing with atomic, molecular, and optical platforms for fundamental physics. Phys. Rev. Lett. 132, 190001 (2024).
Rondin, L. et al. Magnetometry with nitrogen-vacancy defects in diamond. Rep. Prog. Phys. 77, 056503 (2014).
Doherty, M. W. et al. The nitrogen-vacancy colour centre in diamond. Phys. Rep. 528, 1–45 (2013).
Koehl, W. F., Buckley, B. B., Heremans, F. J., Calusine, G. & Awschalom, D. D. Room temperature coherent control of defect spin qubits in silicon carbide. Nature 479, 84–87 (2011).
Widmann, M. et al. Coherent control of single spins in silicon carbide at room temperature. Nat. Mater. 14, 164–168 (2015).
Bejarano, M. et al. Parametric magnon transduction to spin qubits. Sci. Adv. 10, eadi2042 (2024).
Chen, X. et al. Quantum sensing of room-temperature gerromagnetism in 2D van der Waals Fe3GaTe2 using divacancy spins in SiC. Adv. Funct. Mater. 35, 2413529 (2025).
Li, P. et al. Non-invasive bioinert room-temperature quantum sensor from silicon carbide qubits. Nat. Mater. 24, 1913–1919 (2025).
Aharonovich, I., Englund, D. & Toth, M. Solid-state single-photon emitters. Nat. Photon. 10, 631–641 (2016).
Azzam, S. I., Parto, K. & Moody, G. Prospects and challenges of quantum emitters in 2D materials. Appl. Phys. Lett. 118, 240502 (2021).
Gottscholl, A. et al. Initialization and read-out of intrinsic spin defects in a van der Waals crystal at room temperature. Nat. Mater. 19, 540–545 (2020).
Vaidya, S., Gao, X., Dikshit, S., Aharonovich, I. & Li, T. Quantum sensing and imaging with spin defects in hexagonal boron nitride. Adv. Phys. X 8, 2206049 (2023).
Rose, B. C. et al. Observation of an environmentally insensitive solid-state spin defect in diamond. Science 361, 60–63 (2018).
Maletinsky, P. et al. A robust scanning diamond sensor for nanoscale imaging with single nitrogen-vacancy centres. Nat. Nanotechnol. 7, 320–324 (2012).
Gross, I. et al. Real-space imaging of non-collinear antiferromagnetic order with a single-spin magnetometer. Nature 549, 252–256 (2017).
Pelliccione, M. et al. Scanned probe imaging of nanoscale magnetism at cryogenic temperatures with a single-spin quantum sensor. Nat. Nanotechnol. 11, 700–705 (2016).
Song, T. et al. Direct visualization of magnetic domains and moiré magnetism in twisted 2D magnets. Science 374, 1140–1144 (2021).
Tan, A. K. C. et al. Revealing emergent magnetic charge in an antiferromagnet with diamond quantum magnetometry. Nat. Mater. 23, 205–211 (2024).
Li, S. et al. Observation of stacking engineered magnetic phase transitions within moiré supercells of twisted van der Waals magnets. Nat. Commun. 15, 5712 (2024).
Huxter, W. S., Sarott, M. F., Trassin, M. & Degen, C. L. Imaging ferroelectric domains with a single-spin scanning quantum sensor. Nat. Phys. 19, 644–648 (2023).
Thiel, L. et al. Quantitative nanoscale vortex imaging using a cryogenic quantum magnetometer. Nat. Nanotechnol. 11, 677–681 (2016).
Scholten, S. C. et al. Widefield quantum microscopy with nitrogen-vacancy centers in diamond: strengths, limitations, and prospects. J. Appl. Phys. 130, 150902 (2021).
Finco, A. et al. Imaging non-collinear antiferromagnetic textures via single spin relaxometry. Nat. Commun. 12, 767 (2021).
Kolkowitz, S. et al. Probing Johnson noise and ballistic transport in normal metals with a single-spin qubit. Science 347, 1129–1132 (2015).
McCullian, B. A. et al. Broadband multi-magnon relaxometry using a quantum spin sensor for high frequency ferromagnetic dynamics sensing. Nat. Commun. 11, 5229 (2020).
van der Sar, T., Casola, F., Walsworth, R. & Yacoby, A. Nanometre-scale probing of spin waves using single electron spins. Nat. Commun. 6, 7886 (2015).
Rovny, J. et al. Nanoscale covariance magnetometry with diamond quantum sensors. Science 378, 1301–1305 (2022).
Huxter, W. S. et al. Scanning gradiometry with a single spin quantum magnetometer. Nat. Commun. 13, 3761 (2022).
Qiu, Z., Hamo, A., Vool, U., Zhou, T. X. & Yacoby, A. Nanoscale electric field imaging with an ambient scanning quantum sensor microscope. npj Quantum Inf. 8, 107 (2022).
Shields, B. J., Unterreithmeier, Q. P., de Leon, N. P., Park, H. & Lukin, M. D. Efficient readout of a single spin state in diamond via spin-to-charge conversion. Phys. Rev. Lett. 114, 136402 (2015).
Hopper, D. A., Shulevitz, H. J. & Bassett, L. C. Spin readout techniques of the nitrogen-vacancy center in diamond. Micromachines 9, 437 (2018).
Laraoui, A. et al. Imaging thermal conductivity with nanoscale resolution using a scanning spin probe. Nat. Commun. 6, 8954 (2015).
Lesik, M. et al. Magnetic measurements on micrometer-sized samples under high pressure using designed NV centers. Science 366, 1359–1362 (2019).
Yip, K. Y. et al. Measuring magnetic field texture in correlated electron systems under extreme conditions. Science 366, 1355–1359 (2019).
Hsieh, S. et al. Imaging stress and magnetism at high pressures using a nanoscale quantum sensor. Science 366, 1349–1354 (2019).
Bhattacharyya, P. et al. Imaging the Meissner effect in hydride superconductors using quantum sensors. Nature 627, 73–79 (2024).
Broadway, D. A. et al. Imaging domain reversal in an ultrathin van der Waals ferromagnet. Adv. Mater. 32, 2003314 (2020).
Li, Y. et al. Critical fluctuations and noise spectra in two-dimensional Fe3GeTe2 magnets. Nat. Commun. 16, 8585 (2025).
Huang, M. et al. Revealing intrinsic domains and fluctuations of moiré magnetism by a wide-field quantum microscope. Nat. Commun. 14, 5259 (2023).
Melendez, A. L. et al. Quantum sensing of broadband spin dynamics and magnon transport in antiferromagnets. Sci. Adv. 11, eadu9381 (2025).
Schlussel, Y. et al. Wide-field imaging of superconductor vortices with electron spins in diamond. Phys. Rev. Appl. 10, 034032 (2018).
Liu, Z. et al. Quantum noise spectroscopy of superconducting dynamics in thin film Bi2Sr2CaCu2O8+δ. Preprint at https://arxiv.org/abs/2502.04439 (2025).
Aslam, N. et al. Nanoscale nuclear magnetic resonance with chemical resolution. Science 357, 67–71 (2017).
Glenn, D. R. et al. High-resolution magnetic resonance spectroscopy using a solid-state spin sensor. Nature 555, 351–354 (2018).
Lovchinsky, I. et al. Magnetic resonance spectroscopy of an atomically thin material using a single-spin qubit. Science 355, 503–507 (2017).
Wang, Y.-X. et al. Visualization of bulk and edge photocurrent flow in anisotropic Weyl semimetals. Nat. Phys. 19, 507–514 (2023).
Bourgeois, E. et al. Photoelectric detection of electron spin resonance of nitrogen-vacancy centres in diamond. Nat. Commun. 6, 8577 (2015).
Zhou, B. B. et al. Spatiotemporal mapping of a photocurrent vortex in monolayer MoS2 using diamond quantum sensors. Phys. Rev. X 10, 011003 (2020).
Zhang, X.-Y. et al. ac Susceptometry of 2D van der Waals magnets enabled by the coherent control of quantum sensors. PRX Quantum 2, 030352 (2021).
Dasika, S., Markham, M. L. & Saha, K. Quantum diamond microscope method to determine AC susceptibility in micro-magnets. EPJ Quantum. Technol. 12, 85 (2025).
Kehayias, P. et al. Imaging crystal stress in diamond using ensembles of nitrogen-vacancy centers. Phys. Rev. B 100, 174103 (2019).
Trusheim, M. E. & Englund, D. Wide-field strain imaging with preferentially aligned nitrogen-vacancy centers in polycrystalline diamond. New J. Phys. 18, 123023 (2016).
MacQuarrie, E. R., Gosavi, T. A., Jungwirth, N. R., Bhave, S. A. & Fuchs, G. D. Mechanical spin control of nitrogen-vacancy venters in diamond. Phys. Rev. Lett. 111, 227602 (2013).
Balasubramanian, G. et al. Nanoscale imaging magnetometry with diamond spins under ambient conditions. Nature 455, 648–651 (2008).
Tetienne, J.-P. et al. Nanoscale imaging and control of domain-wall hopping with a nitrogen-vacancy center microscope. Science 344, 1366–1369 (2014).
Hingant, T. et al. Measuring the magnetic moment density in patterned ultrathin ferromagnets with submicrometer resolution. Phys. Rev. Appl. 4, 014003 (2015).
Xu, Z. et al. Minimizing sensor-sample distances in scanning nitrogen-vacancy magnetometry. ACS Nano 19, 8255–8265 (2025).
Jelezko, F., Gaebel, T., Popa, I., Gruber, A. & Wrachtrup, J. Observation of coherent oscillations in a single electron spin. Phys. Rev. Lett. 92, 076401 (2004).
Hanson, R., Dobrovitski, V. V., Feiguin, A. E., Gywat, O. & Awschalom, D. D. Coherent dynamics of a single spin interacting with an adjustable spin bath. Science 320, 352–355 (2008).
Wolfe, C. S. et al. Off-resonant manipulation of spins in diamond via precessing magnetization of a proximal ferromagnet. Phys. Rev. B 89, 180406 (2014).
Du, C. et al. Control and local measurement of the spin chemical potential in a magnetic insulator. Science 357, 195–198 (2017).
Jarmola, A., Acosta, V. M., Jensen, K., Chemerisov, S. & Budker, D. Temperature- and magnetic-field-dependent longitudinal spin relaxation in nitrogen-vacancy ensembles in diamond. Phys. Rev. Lett. 108, 197601 (2012).
Ariyaratne, A., Bluvstein, D., Myers, B. A. & Jayich, A. C. B. Nanoscale electrical conductivity imaging using a nitrogen-vacancy center in diamond. Nat. Commun. 9, 2406 (2018).
Dolde, F. et al. Electric-field sensing using single diamond spins. Nat. Phys. 7, 459–463 (2011).
Yang, B. et al. Vector electrometry in a wide-gap-semiconductor device using a spin-ensemble quantum sensor. Phys. Rev. Appl. 14, 044049 (2020).
Li, R. et al. Nanoscale electrometry based on a magnetic-field-resistant spin sensor. Phys. Rev. Lett. 124, 247701 (2020).
Bian, K. et al. Nanoscale electric-field imaging based on a quantum sensor and its charge-state control under ambient condition. Nat. Commun. 12, 2457 (2021).
Mittiga, T. et al. Imaging the local charge environment of nitrogen-vacancy centers in diamond. Phys. Rev. Lett. 121, 246402 (2018).
Palm, M. L. et al. Observation of current whirlpools in graphene at room temperature. Science 384, 465–469 (2024).
Ku, M. J. H. et al. Imaging viscous flow of the Dirac fluid in graphene. Nature 583, 537–541 (2020).
Jenkins, A. et al. Imaging the breakdown of Ohmic transport in graphene. Phys. Rev. Lett. 129, 087701 (2022).
Andersen, T. I. et al. Electron-phonon instability in graphene revealed by global and local noise probes. Science 364, 154–157 (2019).
Monge, R. et al. Spin dynamics of a solid-state qubit in proximity to a superconductor. Nano Lett. 23, 422–428 (2023).
Li, S. et al. Nanoscale observation and control of quasiparticle induced magnetic noise in a superconducting resonator. Phys. Rev. Lett. 136, 076004 (2026).
Acosta, V. M. et al. Temperature dependence of the nitrogen-vacancy magnetic resonance in diamond. Phys. Rev. Lett. 104, 070801 (2010).
Kucsko, G. et al. Nanometre-scale thermometry in a living cell. Nature 500, 54–58 (2013).
Wang, N. et al. Magnetic criticality enhanced hybrid nanodiamond thermometer under ambient conditions. Phys. Rev. X 8, 011042 (2018).
Toyli, D. M., de las Casas, C. F., Christle, D. J., Dobrovitski, V. V. & Awschalom, D. D. Fluorescence thermometry enhanced by the quantum coherence of single spins in diamond. Proc. Natl Acad. Sci. USA 110, 8417–8421 (2013).
Doherty, M. W. et al. Electronic properties and metrology applications of the diamond NV− center under pressure. Phys. Rev. Lett. 112, 047601 (2014).
Steele, L. G. et al. Optically detected magnetic resonance of nitrogen vacancies in a diamond anvil cell using designer diamond anvils. Appl. Phys. Lett. 111, 221903 (2017).
Ovartchaiyapong, P., Lee, K. W., Myers, B. A. & Jayich, A. C. B. Dynamic strain-mediated coupling of a single diamond spin to a mechanical resonator. Nat. Commun. 5, 4429 (2014).
Teissier, J., Barfuss, A., Appel, P., Neu, E. & Maletinsky, P. Strain coupling of a nitrogen-vacancy center spin to a diamond mechanical oscillator. Phys. Rev. Lett. 113, 020503 (2014).
Keimer, B. & Moore, J. E. The physics of quantum materials. Nat. Phys. 13, 1045–1055 (2017).
Dovzhenko, Y. et al. Magnetostatic twists in room-temperature skyrmions explored by nitrogen-vacancy center spin texture reconstruction. Nat. Commun. 9, 2712 (2018).
Akhtar, W. et al. Current-induced nucleation and dynamics of skyrmions in a Co-based Heusler alloy. Phys. Rev. Appl. 11, 034066 (2019).
Tetienne, J.-P. et al. The nature of domain walls in ultrathin ferromagnets revealed by scanning nanomagnetometry. Nat. Commun. 6, 6733 (2015).
McLaughlin, N. J. et al. Local control of a single nitrogen-vacancy center by nanoscale engineered magnetic domain wall motion. ACS Nano 17, 25689–25696 (2023).
Thiel, L. et al. Probing magnetism in 2D materials at the nanoscale with single-spin microscopy. Science 364, 973–976 (2019).
Tschudin, M. A. et al. Imaging nanomagnetism and magnetic phase transitions in atomically thin CrSBr. Nat. Commun. 15, 6005 (2024).
Högen, M. et al. Imaging nucleation and propagation of pinned domains in few-layer Fe5–xGeTe2. ACS Nano 17, 16879–16885 (2023).
Wang, Y.-X. et al. Configurable antiferromagnetic domains and lateral exchange bias in atomically thin CrPS4. Nat. Mater. 24, 1414–1423 (2025).
Sfeir, E. et al. Room temperature magnetic vortices in the van der Waals magnet Fe5GeTe2. Phys. Rev. Mater. 9, 114003 (2025).
Burch, K. S., Mandrus, D. & Park, J.-G. Magnetism in two-dimensional van der Waals materials. Nature 563, 47–52 (2018).
Yang, H. et al. Two-dimensional materials prospects for non-volatile spintronic memories. Nature 606, 663–673 (2022).
Gong, C. & Zhang, X. Two-dimensional magnetic crystals and emergent heterostructure devices. Science 363, eaav4450 (2019).
Huang, B. et al. Layer-dependent ferromagnetism in a van der Waals crystal down to the monolayer limit. Nature 546, 270–273 (2017).
Gao, A. et al. An antiferromagnetic diode effect in even-layered MnBi2Te4. Nat. Electron. 7, 751–759 (2024).
Pellet-Mary, C. et al. Lateral exchange bias for Néel-vector control in atomically thin antiferromagnets. Nat. Commun. 16, 9725 (2025).
Balents, L., Dean, C. R., Efetov, D. K. & Young, A. F. Superconductivity and strong correlations in moiré flat bands. Nat. Phys. 16, 725–733 (2020).
Andrei, E. Y. et al. The marvels of moiré materials. Nat. Rev. Mater. 6, 201–206 (2021).
Kennes, D. M. et al. Moiré heterostructures as a condensed-matter quantum simulator. Nat. Phys. 17, 155–163 (2021).
Broadway, D. A. et al. Improved current density and magnetization reconstruction through vector magnetic field measurements. Phys. Rev. Appl. 14, 024076 (2020).
Xu, Y. et al. Coexisting ferromagnetic–antiferromagnetic state in twisted bilayer CrI3. Nat. Nanotechnol. 17, 143–147 (2022).
Xie, H. et al. Twist engineering of the two-dimensional magnetism in double bilayer chromium triiodide homostructures. Nat. Phys. 18, 30–36 (2022).
Cheng, G. et al. Electrically tunable moiré magnetism in twisted double bilayers of chromium triiodide. Nat. Electron. 6, 434–442 (2023).
Sivadas, N. et al. Stacking-dependent magnetism in Bilayer CrI3. Nano Lett. 18, 7658–7664 (2018).
Hejazi, K., Luo, Z.-X. & Balents, L. Noncollinear phases in moiré magnets. Proc. Natl Acad. Sci. USA 117, 10721–10726 (2020).
Wong, K. C. et al. Super-moiré spin textures in twisted antiferromagnets. Nat. Nanotechnol. 21, 359–365 (2026).
Finco, A. & Jacques, V. Single spin magnetometry and relaxometry applied to antiferromagnetic materials. APL Mater. 11, 100901 (2023).
Hedrich, N. et al. Nanoscale mechanics of antiferromagnetic domain walls. Nat. Phys. 17, 574–577 (2021).
Appel, P. et al. Nanomagnetism of magnetoelectric granular thin-film antiferromagnets. Nano Lett. 19, 1682–1687 (2019).
Erickson, A. et al. Nanoscale imaging of antiferromagnetic domains in epitaxial films of Cr2O3 via scanning diamond magnetic probe microscopy. RSC Adv. 13, 178–185 (2023).
Wörnle, M. S. et al. Coexistence of Bloch and Néel walls in a collinear antiferromagnet. Phys. Rev. B 103, 094426 (2021).
Li, S. et al. Nanoscale magnetic domains in polycrystalline Mn3Sn films imaged by a scanning single-spin magnetometer. Nano Lett. 23, 5326–5333 (2023).
Tsukamoto, M. et al. Observation of chiral domain walls in an octupole-ordered antiferromagnet. Phys. Rev. B 112, L020404 (2025).
Guo, Q. et al. Current-induced switching of thin film Fe2O3 devices imaged using a scanning single-spin microscope. Phys. Rev. Mater. 7, 064402 (2023).
Meisenheimer, P. et al. Switching the spin cycloid in BiFeO3 with an electric field. Nat. Commun. 15, 2903 (2024).
Jayaram, S. Probing vortex dynamics in 2D superconductors with scanning quantum microscope. Phys. Rev. Lett. 135, 126001 (2025).
Chen, S. et al. Current induced hidden states in Josephson junctions. Nat. Commun. 15, 8059 (2024).
Vool, U. et al. Imaging phonon-mediated hydrodynamic flow in WTe2. Nat. Phys. 17, 1216–1220 (2021).
Scheidegger, P. J., Diesch, S., Palm, M. L. & Degen, C. L. Scanning nitrogen-vacancy magnetometry down to 350 mK. Appl. Phys. Lett. 120, 224001 (2022).
Bradley, C. E. et al. A ten-qubit solid-state spin register with quantum memory up to one minute. Phys. Rev. X 9, 031045 (2019).
Simon, B. G. et al. Directional excitation of a high-density magnon gas using coherently driven spin waves. Nano Lett. 21, 8213–8219 (2021).
Zhou, T. X. et al. A magnon scattering platform. Proc. Natl Acad. Sci. USA 118, e2019473118 (2021).
Lan, G. et al. Coherent harmonic generation of magnons in spin textures. Nat. Commun. 16, 1178 (2025).
Borst, M. et al. Observation and control of hybrid spin-wave–Meissner-current transport modes. Science 382, 430–434 (2023).
Appel, P., Ganzhorn, M., Neu, E. & Maletinsky, P. Nanoscale microwave imaging with a single electron spin in diamond. New J. Phys. 17, 112001 (2015).
Flebus, B. & Tserkovnyak, Y. Quantum-impurity relaxometry of magnetization dynamics. Phys. Rev. Lett. 128, 259901 (2022).
McLaughlin, N. J. et al. Quantum imaging of magnetic phase transitions and spin fluctuations in intrinsic magnetic topological nanoflakes. Nano Lett. 22, 5810–5817 (2022).
Huang, M. et al. Layer-dependent magnetism and spin fluctuations in atomically thin van der Waals magnet CrPS4. Nano Lett. 23, 8099–8105 (2023).
Xue, R. et al. Magnon hydrodynamics in an atomically-thin ferromagnet. Science 392, 873–878 (2026).
Ziffer, M. E. et al. Quantum noise spectroscopy of criticality in an atomically thin magnet. Preprint at https://arxiv.org/abs/2407.05614 (2024).
Sun, Z. et al. Dimensionality crossover to a two-dimensional vestigial nematic state from a three-dimensional antiferromagnet in a honeycomb van der Waals magnet. Nat. Phys. 20, 1764–1771 (2024).
Finco, A. et al. Thermal spin wave noise as a probe for the Dzyaloshinkii–Moriya interaction. Phys. Rev. Lett. 135, 136703 (2025).
Koerner, C. et al. Frequency multiplication by collective nanoscale spin-wave dynamics. Science 375, 1165–1169 (2022).
Hu, Z. et al. Nonlinear magnetic sensing with hybrid nitrogen-vacancy/magnon systems. Nano Lett. 24, 15731–15737 (2024).
Wang, H. et al. Noninvasive measurements of spin transport properties of an antiferromagnetic insulator. Sci. Adv. 8, eabg8562 (2022).
Tschirhart, C. L. et al. Imaging orbital ferromagnetism in a moiré Chern insulator. Science 372, 1323–1327 (2021).
Redekop, E. et al. Direct magnetic imaging of fractional Chern insulators in twisted MoTe2 with a superconducting sensor. Nature 635, 584–589 (2024).
Tschirhart, C. L. et al. Intrinsic spin Hall torque in a moiré Chern magnet. Nat. Phys. 19, 807–813 (2023).
Grinolds, M. S. et al. Nanoscale magnetic imaging of a single electron spin under ambient conditions. Nat. Phys. 9, 215–219 (2013).
Grover, S. et al. Chern mosaic and Berry-curvature magnetism in magic-angle graphene. Nat. Phys. 18, 885–892 (2022).
Ye, M., Seo, H. & Galli, G. Spin coherence in two-dimensional materials. npj Comput. Mater. 5, 44 (2019).
Cai, H. et al. Charge-depletion-enhanced WSe2 quantum emitters on gold nanogap arrays with near-unity quantum efficiency. Nat. Photon. 18, 842–847 (2024).
Vaidya, S. et al. Coherent spins in van der Waals semiconductor GeS2 at ambient conditions. Nano Lett. 25, 14356–14362 (2025).
Healey, A. J. et al. Quantum microscopy with van der Waals heterostructures. Nat. Phys. 19, 87–91 (2023).
Yu, P. et al. Excited-state spectroscopy of spin defects in hexagonal boron nitride. Nano Lett. 22, 3545–3549 (2022).
Mathur, N. et al. Excited-state spin-resonance spectroscopy of \({{\rm{V}}}_{{\rm{B}}}^{-}\) defect centers in hexagonal boron nitride. Nat. Commun. 13, 3233 (2022).
Baber, S. et al. Excited state spectroscopy of boron vacancy defects in hexagonal boron nitride using time-resolved optically detected magnetic resonance. Nano Lett. 22, 461–467 (2022).
Haykal, A. et al. Decoherence of \({{\rm{V}}}_{{\rm{B}}}^{-}\) spin defects in monoisotopic hexagonal boron nitride. Nat. Commun. 13, 4347 (2022).
Gottscholl, A. et al. Spin defects in hBN as promising temperature, pressure and magnetic field quantum sensors. Nat. Commun. 12, 4480 (2021).
Scholten, S. C. et al. Multi-species optically addressable spin defects in a van der Waals material. Nat. Commun. 15, 6727 (2024).
Stern, H. L. et al. A quantum coherent spin in hexagonal boron nitride at ambient conditions. Nat. Mater. 23, 1379–1385 (2024).
Gao, X. et al. Single nuclear spin detection and control in a van der Waals material. Nature 643, 943–949 (2025).
Dean, C. R. et al. Boron nitride substrates for high-quality graphene electronics. Nat. Nanotechnol. 5, 722–726 (2010).
Geim, A. K. & Grigorieva, I. V. Van der Waals heterostructures. Nature 499, 419–425 (2013).
Zhou, J. et al. Sensing spin wave excitations by spin defects in few-layer-thick hexagonal boron nitride. Sci. Adv. 10, eadk8495 (2024).
Durand, A. et al. Optically active spin defects in few-layer thick hexagonal boron nitride. Phys. Rev. Lett. 131, 116902 (2023).
Zhang, X. et al. Visualizing field-free deterministic magnetic switching of all-van der Waals spin–orbit torque system using spin ensembles in hexagonal boron nitride. Nat. Commun. https://doi.org/10.1038/s41467-026-74178-7 (2026).
Huang, M. et al. Wide field imaging of van der Waals ferromagnet Fe3GeTe2 by spin defects in hexagonal boron nitride. Nat. Commun. 13, 5369 (2022).
Kumar, P. et al. Magnetic imaging with spin defects in hexagonal boron nitride. Phys. Rev. Appl. 18, L061002 (2022).
Zhong, C. et al. Ultrasensitive pressure sensing with boron vacancy defects in hexagonal boron nitride: in-situ pressure imaging of two-dimensional heterostructures under high pressure. ACS Photon. 12, 3717–3724 (2025).
Das, S. et al. Quantum sensing of spin dynamics using boron-vacancy centers in hexagonal boron nitride. Phys. Rev. Lett. 133, 166704 (2024).
Zang, H.-X. et al. Detecting and imaging of magnons at nanoscale with van der Waals quantum sensor. Adv. Funct. Mater. 35, 2412166 (2025).
Mañas-Valero, S. et al. Isofrequency spin-wave imaging using color center magnetometry for magnon spintronics. Nat. Commun. 17, 379 (2026).
Mu, Z. et al. Magnetic imaging under high pressure with a spin-based quantum sensor integrated in a van der Waals heterostructure. Nat. Commun. 16, 8574 (2025).
He, G. et al. Probing stress and magnetism at high pressures with two-dimensional quantum sensors. Nat. Commun. 16, 8162 (2025).
Gao, X. et al. Room-temperature quantum entanglement in a van der Waals material. Preprint at https://arxiv.org/abs/2509.23170 (2025).
Robertson, I. O. et al. A charge transfer mechanism for optically addressable solid-state spin pairs. Nat. Phys. 21, 1981–1987 (2025).
Gao, X. et al. Nanotube spin defects for omnidirectional magnetic field sensing. Nat. Commun. 15, 7697 (2024).
Rizzato, R. et al. Quantum sensing with spin defects in boron nitride nanotubes. Nat. Commun. 16, 11333 (2025).
Welter, P. et al. Scanning nitrogen-vacancy center magnetometry in large in-plane magnetic fields. Appl. Phys. Lett. 120, 074003 (2022).
Rohner, D. et al. (111)-oriented, single crystal diamond tips for nanoscale scanning probe imaging of out-of-plane magnetic fields. Appl. Phys. Lett. 115, 192401 (2019).
Appel, P. et al. Fabrication of all diamond scanning probes for nanoscale magnetometry. Rev. Sci. Instrum. 87, 063703 (2016).
Zhu, T. et al. Multicone diamond waveguides for nanoscale quantum sensing. Nano Lett. 23, 10110–10117 (2023).
Wang, M. et al. Self-aligned patterning technique for fabricating high-performance diamond sensor arrays with nanoscale precision. Sci. Adv. 8, eabn9573 (2022).
van Dam, S. B. et al. Optical coherence of diamond nitrogen-vacancy centers formed by ion implantation and annealing. Phys. Rev. B 99, 161203 (2019).
Guo, X. et al. Direct-bonded diamond membranes for heterogeneous quantum and electronic technologies. Nat. Commun. 15, 8788 (2024).
Ohashi, K. et al. Negatively charged nitrogen-vacancy centers in a 5 nm thin 12C diamond film. Nano Lett. 13, 4733–4738 (2013).
Grotz, B. et al. Charge state manipulation of qubits in diamond. Nat. Commun. 3, 729 (2012).
Hauf, M. V. et al. Chemical control of the charge state of nitrogen-vacancy centers in diamond. Phys. Rev. B 83, 081304 (2011).
Hughes, L. B. et al. Strongly interacting, two-dimensional, dipolar spin ensembles in (111)-oriented diamond. Phys. Rev. X 15, 021035 (2025).
Achard, J., Jacques, V. & Tallaire, A. Chemical vapour deposition diamond single crystals with nitrogen-vacancy centres: a review of material synthesis and technology for quantum sensing applications. J. Phys. D 53, 313001 (2020).
McLellan, C. A. et al. Patterned formation of highly coherent nitrogen-vacancy centers using a focused electron irradiation technique. Nano Lett. 16, 2450–2454 (2016).
Hedrich, N., Rohner, D., Batzer, M., Maletinsky, P. & Shields, B. J. Parabolic diamond scanning probes for single-spin magnetic field imaging. Phys. Rev. Appl. 14, 064007 (2020).
Zabelotsky, T. et al. Creation of boron vacancies in hexagonal boron nitride exfoliated from bulk crystals for quantum sensing. ACS Appl. Nano Mater. 6, 21671–21678 (2023).
Herb, K. et al. Quantum magnetometry of transient signals with a time resolution of 1.1 nanoseconds. Nat. Commun. 16, 822 (2025).
Fuchs, G. D., Dobrovitski, V. V., Toyli, D. M., Heremans, F. J. & Awschalom, D. D. Gigahertz dynamics of a strongly driven single quantum spin. Science 326, 1520–1522 (2009).
Yan, G. Q. et al. Coherent driving of a single nitrogen vacancy center by a resonant magnetic tunnel junction. Nano Lett. 24, 14273–14278 (2024).
Yan, G. Q. et al. Electric-field-induced coherent control of nitrogen-vacancy centers. Phys. Rev. Appl. 18, 064031 (2022).
Labanowski, D. et al. Voltage-driven, local, and efficient excitation of nitrogen-vacancy centers in diamond. Sci. Adv. 4, eaat6574 (2018).
Wang, X. et al. Electrical control of coherent spin rotation of a single-spin qubit. npj Quantum Inf. 6, 78 (2020).
Barfuss, A., Teissier, J., Neu, E., Nunnenkamp, A. & Maletinsky, P. Strong mechanical driving of a single electron spin. Nat. Phys. 11, 820–824 (2015).
Zhang, H. et al. Spin-torque oscillation in a magnetic insulator probed by a single-spin sensor. Phys. Rev. B 102, 024404 (2020).
Wolf, M. S., Badea, R. & Berezovsky, J. Fast nanoscale addressability of nitrogen-vacancy spins via coupling to a dynamic ferromagnetic vortex. Nat. Commun. 7, 11584 (2016).
Niknam, M. et al. Quantum control of spin qubits using nanomagnets. Commun. Phys. 5, 284 (2022).
Stepanov, V., Cho, F. H., Abeywardana, C. & Takahashi, S. High-frequency and high-field optically detected magnetic resonance of nitrogen-vacancy centers in diamond. Appl. Phys. Lett. 106, 063111 (2015).
Zuber, J. A. et al. Shallow silicon vacancy centers with lifetime-limited optical linewidths in diamond nanostructures. Nano Lett. 23, 10901–10907 (2023).
Cao, Y. et al. Unconventional superconductivity in magic-angle graphene superlattices. Nature 556, 43–50 (2018).
Hasan, M. Z. & Kane, C. L. Colloquium: topological insulators. Rev. Mod. Phys. 82, 3045–3067 (2010).
Qi, X.-L. & Zhang, S.-C. Topological insulators and superconductors. Rev. Mod. Phys. 83, 1057–1110 (2011).
Burkov, A. A. Topological semimetals. Nat. Mater. 15, 1145–1148 (2016).
Lv, B. Q., Qian, T. & Ding, H. Experimental perspective on three-dimensional topological semimetals. Rev. Mod. Phys. 93, 025002 (2021).
Yan, B. & Felser, C. Topological materials: Weyl semimetals. Annu. Rev. Condens. Matter Phys. 8, 337–354 (2017).
Jia, S., Xu, S.-Y. & Hasan, M. Z. Weyl semimetals, Fermi arcs and chiral anomalies. Nat. Mater. 15, 1140–1144 (2016).
Broholm, C. et al. Quantum spin liquids. Science 367, eaay0668 (2020).
Savary, L. & Balents, L. Quantum spin liquids: a review. Rep. Prog. Phys. 80, 016502 (2016).
Zhou, Y., Kanoda, K. & Ng, T.-K. Quantum spin liquid states. Rev. Mod. Phys. 89, 025003 (2017).
Khoo, J. Y., Pientka, F., Lee, P. A. & Villadiego, I. S. Probing the quantum noise of the spinon Fermi surface with NV centers. Phys. Rev. B 106, 115108 (2022).
Chatterjee, S., Rodriguez-Nieva, J. F. & Demler, E. Diagnosing phases of magnetic insulators via noise magnetometry with spin qubits. Phys. Rev. B 99, 104425 (2019).
Chang, C.-Z. et al. Experimental observation of the quantum anomalous Hall effect in a magnetic topological insulator. Science 340, 167–170 (2013).
Deng, Y. et al. Quantum anomalous Hall effect in intrinsic magnetic topological insulator MnBi2Te4. Science 367, 895–900 (2020).
Ju, L., MacDonald, A. H., Mak, K. F., Shan, J. & Xu, X. The fractional quantum anomalous Hall effect. Nat. Rev. Mater. 9, 455–459 (2024).
Lenz, T. et al. Imaging topological spin structures using light-polarization and magnetic microscopy. Phys. Rev. Appl. 15, 024040 (2021).
Tang, H. et al. On-chip multi-degree-of-freedom control of two-dimensional materials. Nature 632, 1038–1044 (2024).
Aharon-Steinberg, A. et al. Direct observation of vortices in an electron fluid. Nature 607, 74–80 (2022).
Wang, W. et al. Direct evidence of ferromagnetism in a quantum anomalous Hall system. Nat. Phys. 14, 791–795 (2018).
Wu, Y. et al. A van der Waals interface hosting two groups of magnetic skyrmions. Adv. Mater. 34, 2110583 (2022).
Inbar, A. et al. The quantum twisting microscope. Nature 614, 682–687 (2023).